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Hm. I'd have to say Death Note and Higurashi no Naku Koro Ni.
Both of them made me laugh.
Also, they helped me think more about what was goin on behind the scenes of what was apparent

Extremely high pitched voices when the character it belongs to is absolutely useless half of the time.

I agree with the thread starter, but I'm also going to add in Mx0

HAHA Sakura from Naruto, cause she's hella useless the first part of the story, and then the author makes her hella rigged later. Asuka from Neon. Orihime from Bleach. And someone else.